Dense emulsions, colloidal gels, microgels, and foams all display a solidlike behavior at rest characterized by a yield stress, above which the material flows like a liquid. Such a fluidization transition often consists of long-lasting transient flows that involve shear-banded velocity profiles. The characteristic time for full fluidization tau(f) has been reported to decay as a power law of the shear rate (gamma) over dot and of the shear stress sigma with respective exponents alpha and beta. Strikingly, the ratio of these exponents was empirically observed to coincide with the exponent of the Herschel-Bulkley law that describes the steady-state flow behavior of these complex fluids. Here we introduce a continuum model, based on the minimization of a "free energy," that captures quantitatively all the salient features associated with such transient shear banding. More generally, our results provide a unified theoretical framework for describing the yielding transition and the steady-state flow properties of yield stress fluids.
Benzi, R., Divoux, T., Barentin, C., Manneville, S., Sbragaglia, M., Toschi, F. (2019). Unified Theoretical and Experimental View on Transient Shear Banding. PHYSICAL REVIEW LETTERS, 123(24), 248001-248004 [10.1103/PhysRevLett.123.248001].
Unified Theoretical and Experimental View on Transient Shear Banding
Benzi R.Membro del Collaboration Group
;Sbragaglia M.Membro del Collaboration Group
;Toschi F.Membro del Collaboration Group
2019-12-09
Abstract
Dense emulsions, colloidal gels, microgels, and foams all display a solidlike behavior at rest characterized by a yield stress, above which the material flows like a liquid. Such a fluidization transition often consists of long-lasting transient flows that involve shear-banded velocity profiles. The characteristic time for full fluidization tau(f) has been reported to decay as a power law of the shear rate (gamma) over dot and of the shear stress sigma with respective exponents alpha and beta. Strikingly, the ratio of these exponents was empirically observed to coincide with the exponent of the Herschel-Bulkley law that describes the steady-state flow behavior of these complex fluids. Here we introduce a continuum model, based on the minimization of a "free energy," that captures quantitatively all the salient features associated with such transient shear banding. More generally, our results provide a unified theoretical framework for describing the yielding transition and the steady-state flow properties of yield stress fluids.File | Dimensione | Formato | |
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